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Light absorption characteristics of carbonaceous aerosols in two remote stations of the southern fringe of the Tibetan Plateau, China
Li, CL (Li, Chaoliu)1,3; Yan, FP (Yan, Fangping)2; Kang, SC (Kang, Shichang)2,3; Chen, PF (Chen, Pengfei)2; Hu, ZF (Hu, Zhaofu)2,4; Gao, SP (Gao, Shaopeng)1; Qu, B (Qu, Bin)5; Sillanpaa, M (Sillanpaa, Mika)5,6; Li, CL
Source PublicationATMOSPHERIC ENVIRONMENT
2016
Volume143Issue:0Pages:79-85
DOI10.1016/j.atmosenv.2016.08.042
AbstractLight absorption characteristics of carbonaceous aerosols are key considerations in climate forcing research. However, in situ measurement data are limited, especially on the Tibetan Plateau (TP) - the Third Pole of the world. In this study, the mass absorption cross section (MAC) of elemental carbon (EC) and water soluble organic carbon (WSOC) of total suspended particles at two high-altitude stations (Lulang station and Everest station) in the Tibetan Plateau (TP) were investigated. The mean MAC(EC) values at 632 nm were 6.85 +/- 1.39 m(2) g(-1) and 6.49 +/- 2.81 m(2) g(-1) at these two stations, both of which showed little seasonal variations and were slightly higher than those of EC of uncoated particles, indicating that the enhancement of MAC(EC) by factors such as coating with organic aerosols was not significant. The mean MAC(WSOC) values at 365 nm were 0.84 +/- 0.40 m(2) g(-1) and 1.18 +/- 0.64 m(2) g(-1) at the two stations. Obvious seasonal variations of high and low MACwsoc values appeared in winter and summer, respectively, mainly reflecting photobleaching of light absorption components of WSOC caused by fluctuations in sunlight intensity. Therefore, this phenomenon might also exists in other remote areas of the world. The relative contributions of radiative forcing of WSOC to EC were 6.03 +/- 3.62% and 11.41 +/- 7.08% at these two stations, with a higher ratio in winter. As a result, both the contribution of WSOC to radiative forcing of carbonaceous aerosols and its seasonal variation need to be considered in radiative forcing related study. (C) 2016 Elsevier Ltd. All rights reserved.
Subject Area自然地理学
WOS IDWOS:000383932400008
Language英语
Indexed BySCI
KeywordSoluble Organic-carbon Nam Co Region 5079 m A.s.l. Black Carbon Brown Carbon Chemical Characteristics Source Apportionment Optical-properties Elemental Carbon Lhasa City
Cooperation Status国际
Department环境
SubtypeArticle
Citation statistics
Document Type期刊论文
Identifierhttp://ir.itpcas.ac.cn/handle/131C11/7594
Collection图书馆
Corresponding AuthorLi, CL
Affiliation1.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China
2.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Peoples R China
3.Chinese Acad Sci, CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
5.Lappeenranta Univ Technol, Lab Green Chem, Sammonkatu 12, FI-50130 Mikkeli, Finland
6.Florida Int Univ, Dept Civil & Environm Engn, Miami, FL 33174 USA
Recommended Citation
GB/T 7714
Li, CL ,Yan, FP ,Kang, SC ,et al. Light absorption characteristics of carbonaceous aerosols in two remote stations of the southern fringe of the Tibetan Plateau, China[J]. ATMOSPHERIC ENVIRONMENT,2016,143(0):79-85.
APA Li, CL .,Yan, FP .,Kang, SC .,Chen, PF .,Hu, ZF .,...&Li, CL.(2016).Light absorption characteristics of carbonaceous aerosols in two remote stations of the southern fringe of the Tibetan Plateau, China.ATMOSPHERIC ENVIRONMENT,143(0),79-85.
MLA Li, CL ,et al."Light absorption characteristics of carbonaceous aerosols in two remote stations of the southern fringe of the Tibetan Plateau, China".ATMOSPHERIC ENVIRONMENT 143.0(2016):79-85.
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