Water-Soluble Brown Carbon in Atmospheric Aerosols from Godavari (Nepal), a Regional Representative of South Asia | |
Wu, GM (Wu, Guangming1; Ram, K (Ram, Kirpa)1,2; Fu, PQ (Fu, Pingqing)3; Wang, W (Wang, Wan)4; Zhang, YL (Zhang, Yanlin)5; Liu, XY (Liu, Xiaoyan)5; Stone, EA (Stone, Elizabeth A.)6; Pradhan, BB (Pradhan, Bidya Banmali)7; Dangol, PM (Dangol, Pradeep Man)7; Panday, AK (Panday, Arnico K.)7; Wan, X (Wan, Xin)1,10; Bai, ZP (Bai, Zhipeng)4; Kang, SC (Kang, Shichang)8,9; Zhang, QG (Zhang, Qianggong)1,9; Cong, ZY (Cong, Zhiyuan)1,9 | |
Source Publication | ENVIRONMENTAL SCIENCE & TECHNOLOGY |
2019 | |
Volume | 53Issue:7Pages:3471-3479 |
DOI | 10.1021/acs.est.9b00596 |
Abstract | Brown carbon (BrC) has recently emerged as an important light-absorbing aerosol. This study provides interannual and seasonal variations in light absorption properties, chemical composition, and sources of water-soluble BrC (WS-BrC) based on PM10 samples collected in Godavari, Nepal, from April 2012 to May 2014. The mass absorption efficiency of WS-BrC at 365 nm (MAE(365)) shows a clear seasonal variability, with the highest MAE(365) of 1.05 +/- 0.21 m(2) g(-1) in premonsoon season and the lowest in monsoon season (0.59 +/- 0.16 m(2) g(-1)). The higher MAE(365) values in nonmonsoon seasons are associated with fresh biomass burning emissions. This is further substantiated by a strong correlation (r = 0.79, P < 0.01) between Abs(365) (light absorption coefficient at 365 nm) and levoglucosan. We found, using fluorescence techniques, that humic-like and protein-like substances are the main chromophores in WS-BrC and responsible for 80.2 +/- 4.1% and 19.8 +/- 4.1% of the total fluorescence intensity, respectively. BrC contributes to 8.78 +/- 3.74% of total light absorption over the 300-700 nm wavelength range. Considering the dominant contribution of biomass burning to BrC over Godavari, this study suggests that reduction in biomass burning emission may be a practical method for climate change mitigation in South Asia. |
Subject Area | Environmental Sciences |
WOS ID | WOS:000463679600014 |
Language | 英语 |
Indexed By | SCI |
Keyword | Light-absorption Properties Chemical-composition Source Apportionment Organic Aerosols Black Carbon Biomass Fluorescence Pm2.5 Pm10 Particles |
WOS Research Area | Engineering ; Environmental Sciences & Ecology |
WOS Subject | Engineering, Environmental ; Environmental Sciences |
Cooperation Status | 国际 |
ISSN | 0013-936X |
Department | 环境变化与地表过程 |
URL | 查看原文 |
Publisher | AMER CHEMICAL SOC |
Subtype | Article |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.itpcas.ac.cn/handle/131C11/9338 |
Collection | 图书馆 |
Corresponding Author | Cong, ZY (Cong, Zhiyuan) |
Affiliation | 1.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China; 2.Banaras Hindu Univ, Inst Environm & Sustainable Dev, Varanasi 221005, Uttar Pradesh, India; 3.Tianjin Univ, Inst Surface Earth Syst Sci, Tianjin 300072, Peoples R China; 4.Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China; 5.Nanjing Univ Informat Sci & Technol, Yale NUIST Ctr Atmospher Environm, Nanjing 210044, Jiangsu, Peoples R China; 6.Univ Iowa, Dept Chem, Iowa City, IA 52246 USA; 7.Int Ctr Integrated Mt Dev, Khumaltar 009771, Lalitpur, Nepal; 8.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Cryospher Sci, Lanzhou 730000, Gansu, Peoples R China; 9.Chinese Acad Sci, Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China; 10.Univ Chinese Acad Sci, Beijing 100049, Peoples R China. |
Recommended Citation GB/T 7714 | Wu, GM (Wu, Guangming,Ram, K ,Fu, PQ ,et al. Water-Soluble Brown Carbon in Atmospheric Aerosols from Godavari (Nepal), a Regional Representative of South Asia[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2019,53(7):3471-3479. |
APA | Wu, GM .,Ram, K .,Fu, PQ .,Wang, W .,Zhang, YL .,...&Cong, ZY .(2019).Water-Soluble Brown Carbon in Atmospheric Aerosols from Godavari (Nepal), a Regional Representative of South Asia.ENVIRONMENTAL SCIENCE & TECHNOLOGY,53(7),3471-3479. |
MLA | Wu, GM ,et al."Water-Soluble Brown Carbon in Atmospheric Aerosols from Godavari (Nepal), a Regional Representative of South Asia".ENVIRONMENTAL SCIENCE & TECHNOLOGY 53.7(2019):3471-3479. |
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