| Source appointment of fine particle number and volume concentration during severe haze pollution in Beijing in January 2013 | |
| Liu, ZR (Liu, Zirui)1; Wang, YS (Wang, Yuesi)1; Hu, B (Hu, Bo)1; Ji, DS (Ji, Dongsheng)1; Zhang, JK (Zhang, Junke)1; Wu, FK (Wu, Fangkun)1; Wan, X (Wan, Xin)2; Wang, YH (Wang, Yonghong)3; Wang, YS | |
| Source Publication | ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
 |
| 2016 | |
| Volume | 23Issue:7Pages:6845-6860 |
| DOI | 10.1007/s11356-015-5868-6 |
| Abstract | Extreme haze episodes repeatedly shrouded Beijing during the winter of 2012-2013, causing major environmental and health problems. To better understand these extreme events, particle number size distribution (PNSD) and particle chemical composition (PCC) data collected in an intensive winter campaign in an urban site of Beijing were used to investigate the sources of ambient fine particles. Positive matrix factorization (PMF) analysis resolved a total of eight factors: two traffic factors, combustion factors, secondary aerosol, two accumulation mode aerosol factors, road dust, and long-range transported (LRT) dust. Traffic emissions (54 %) and combustion aerosol (27 %) were found to be the most important sources for particle number concentration, whereas combustion aerosol (33 %) and accumulation mode aerosol (37 %) dominated particle volume concentrations. Chemical compositions and sources of fine particles changed dynamically in the haze episodes. An enhanced role of secondary inorganic species was observed in the formation of haze pollution. Regional transport played an important role for high particles, contribution of which was on average up to 24-49 % during the haze episodes. Secondary aerosols from urban background presented the largest contributions (45 %) for the rapid increase of fine particles in the severest haze episode. In addition, the invasion of LRT dust aerosols further elevated the fine particles during the extreme haze episode. Our results showed a clear impact of regional transport on the local air pollution, suggesting the importance of regional-scale emission control measures in the local air quality management of Beijing. |
| Subject Area | 自然地理学 |
| WOS ID | WOS:000373632400079 |
| Language | 英语 |
| Indexed By | SCI |
| Keyword | Positive Matrix Factorization Size-distribution Data Biomass Burning Contribution Source Apportionment Particulate Matter Air-pollution Eastern China United-states Regional Haze Major Highway |
| Cooperation Status | 国内 |
| Department | 环境 |
| Subtype | Article |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.itpcas.ac.cn/handle/131C11/7722 |
| Collection | 图书馆 |
| Corresponding Author | Wang, YS |
| Affiliation | 1.Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China 2.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100085, Peoples R China 3.Lanzhou Univ, Coll Atmospher Sci, Lanzhou 730000, Peoples R China |
| Recommended Citation GB/T 7714 | Liu, ZR ,Wang, YS ,Hu, B ,et al. Source appointment of fine particle number and volume concentration during severe haze pollution in Beijing in January 2013[J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,2016,23(7):6845-6860. |
| APA | Liu, ZR .,Wang, YS .,Hu, B .,Ji, DS .,Zhang, JK .,...&Wang, YS.(2016).Source appointment of fine particle number and volume concentration during severe haze pollution in Beijing in January 2013.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,23(7),6845-6860. |
| MLA | Liu, ZR ,et al."Source appointment of fine particle number and volume concentration during severe haze pollution in Beijing in January 2013".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH 23.7(2016):6845-6860. |
| Files in This Item: | ||||||
| File Name/Size | DocType | Version | Access | License | ||
| V.23(7) 6845-6860 20（1002KB） | 期刊论文 | 作者接受稿 | 开放获取 | CC BY-NC-SA | View Application Full Text | |
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